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围绕建筑节能、储能与能源转化器件领域中低成本合成与结构稳定控制、表界面结构调控、纳米功能性精准设计等科学难题和技术瓶颈，开展了氧化钨基气致变色薄膜、氧化钒基电极、高性能电催化新材料低成本合成、氧空位产生与表面修饰和构效关系的精确理论设计等工作。针对高表面纳米材料表面氧空位的精确控制，自主开发了表面氧空位控制的原位真空气相包覆设备。针对下一代建筑节能窗体，完成了气致变色智能窗系统产业化技术攻关和示范。以第一(共同)作者和通讯作者(共同)身份在Advanced Materials、Nature Communications、Advanced Functional Materials、Energy Storage Materials等国内外高影响力期刊发表SCI论文60余篇，其中包含ESI高倍引用论文2篇，ESI热门引用论文1篇，SCI他引次数达到3800余次。出版专著1部，授权国家发明专利11项。主持国家自然科学基金面上项目两项、国际合作项目一项、联合资助基金重点项目(二级课题主持)一项。
1. Wen, Y.; Wang, T.; Hao, J.; Zhuang, Z.; Gao, G.; Lai, F.; Lu, S.; Wang, X.; Kang, Q.; Wu, G.; Du, M.; Zhu, H., A CoherentPd-Pd16B3 Core-ShellElectrocatalyst for Controlled Hydrogenation in Nitrogen Reduction Reaction. Adv Funct Mater 2024, 34 (34).
2. Liu, Y.; Wang, T.; Zhang, M.; Gao, G.; Yang, J.; Cai, K., Fastand efficient in-situ construction of low crystalline PEDOT-intercalated V2O5nanosheets for high-performance zinc-ion battery. Chem. Eng. J. 2024, 484.
3. Hao, J.; Wang, T.; Yu, R.; Cai, J.; Gao, G.; Zhuang, Z.; Kang, Q.; Lu, S.; Liu, Z.; Wu, J.; Wu, G.; Du, M.; Wang, D.; Zhu, H., Integrating few-atom layer metal on high-entropyalloys to catalyze nitrate reduction in tandem. Nat Commun 2024, 15 (1), 9020-9020.
4. Deng, S. Y.; Li, J.W.; Zewdie, G. M.; Jiang, X. D.; Ji, M. Z.; Shen, J.; Gao, G. H.; Wu, G. M.; Bao, Z. H.; Kang, H.S., Mg-Doped Porous Silicon Derived from Silica Aerogels for Fast and StableZinc-Ion Hybrid Capacitors with High Capacitance. Adv Funct Mater 2024, 34 (13), 11.
5. Bi, W.; Li, S.; Wang, W.; Liu, Y.; Shen, J.; Gao, G.; Zhang, Z.; Wu, G.; Cao, G., MXenesand their composites as electrodes for sodium ion batteries. Energy Storage Mater 2024, 71.
6. Sun, L.; Zheng, W.; Kang, F.; Gao, W.; Wang, T.; Gao, G.; Xu, W., On-surface synthesis andcharacterization of anti-aromatic cyclo 12 carbon and cyclo 20 carbon. Nat Commun 2024, 15 (1).
7. Yan, W.; Chen, J.; Wang, T.; Mateen, A.; Tang, L.; Sun, S.; Jin, C.; Li, J.; Li, H.; Chen, J.; Gao, G.; Wu, G.; Kang, H. S.; Bao, Z., Orbital interactions and high spin states:Unlocking the potential of Co-Single-Atom catalysts for Li-S batteries. Chem. Eng. J. 2024, 497.
8. Hao, J.; Wang, T.; Cai, J.; Gao, G.; Zhuang, Z.; Yu, R.; Wu, J.; Wu, G.; Lu, S.; Wang, X.; Du, M.; Wang, D.; Zhu, H., Suppression of StructuralHeterogeneity in High-Entropy Intermetallics for Electrocatalytic Upgrading ofWaste Plastics. Angewandte Chemie(International ed. in English) 2024,e202419369-e202419369.
9. Bi, W. C.; Gao, G.H.; Li, C.; Wu, G. M.; Cao, G. Z., Synthesis, properties,and applications of MXenes and their composites for electrical energy storage. Prog. Mater. Sci. 2024, 142, 56.
10. Yin, Q.; Wang, T. D.; Song, Z. H.; Yang, S. H.; Miao, Y. D.; Wu, Y. J.; Sui, Y. W.; Qi, J. Q.; Li, Y. Z.; Zhao, D. Y.; Gao, G. H.; Han, J.B., Computational high-throughput screening of layered double hydroxides ascathodes for chloride ion batteries. Chem.Eng. J. 2023, 459.
11. Zhu, H.; Sun, S. H.; Hao, J. C.; Zhuang, Z. C.; Zhang, S. G.; Wang, T. D.; Kang, Q.; Lu, S. L.; Wang, X. F.; Lai, F. L.; Liu, T. X.; Gao, G. H.; Du, M. L.; Wang, D. S., A high-entropy atomic environment convertsinactive to active sites for electrocatalysis. Energy & Environmental Science 2023, 16 (2), 619-628.
12. Jiang, X. D.; Ji, M.Z.; Gao, G. H.; Yan, X.; Xu, Z.; Bi, W. C.; Cheng, Q.; Wu, G. M., High-ModulusModifications: Stress-Resilient Electrode Materials for Stable Lithium-IonBatteries. Phys Rev Appl 2023, 20 (2).
13. Ji, M. Z.; Ni, J.; Liang, X.; Cheng, Q.; Gao, G. H.; Wu, G. M.; Xiao, Q. F., Biomimetic Synthesisof VO<sub>x</sub>@C Yolk-Shell Nanospheres and Their Application inLi-S Batteries. Adv Funct Mater 2022, 32 (48), 12.
14. Bi, W. C.; Deng, S.Y.; Tang, H. S.; Liu, Y.; Shen, J.; Gao, G. H.; Wu, G. M.; Atif, M.; AlSalhi, M. S.; Gao, G.Z., Coherent V<SUP>4+</SUP>-richV<sub>2</sub>O<sub>5</sub>/carbon aerogelnanocomposites for high performance supercapacitors. Sci China Mater 2022, 65 (7), 1797-1804.
15. Dou, Y. B.; Yao, Y.C.; Wu, G. G.; Gao, G. H.; Zatloukal, M.; Hélix-Nielsen, C.;Zhang, W. J., A defect-rich layered double hydroxide nanofiber filter withsolar-driven regeneration for wastewater treatment. Chem. Eng. J. 2022, 430, 9.
16. Bi, W. C.; Jiang, X.D.; Li, C.; Liu, Y.; Gao, G. H.; Wu, G. M.; Atif, M.; AlSalhi, M.; Cao, G. Z., Effects of Valence States of Working Cations onthe Electrochemical Performance of Sodium Vanadate. Acs Appl Mater Inter 2022,14 (17), 19714-19724.
17. Yuan, F.; Gao, G. H.; Jiang, X. D.; Bi, W. C.; Su, Y. X.; Guo, J. W.; Bao, Z. H.; Shen, J.; Wu, G. M.,Suppressing the metal-metal interaction byCoZn<sub>0.5</sub>V<sub>1.5</sub>O<sub>4</sub>derived from two-dimensional metal-organic frameworks for supercapacitors. Sci China Mater 2022, 65 (1), 105-114.
18. Hao, J. C.; Zhuang, Z.C.; Cao, K. C.; Gao, G. H.; Wang, C.; Lai, F. L.; Lu, S. L.; Ma, P. M.; Dong, W. F.; Liu, T. X.; Du, M. L.; Zhu, H., Unraveling the electronegativity-dominatedintermediate adsorption on high-entropy alloy electrocatalysts. Nat Commun 2022, 13 (1).
19. Guo, M.; Wang, J.; Dou, H.; Gao, G.; Wang, S.; Wang, J.; Xiao, Z.; Wu, G.; Yang, X.; Ma, Z.-F., Agglomeration-resistant2D nanoflakes configured with super electronic networks for extraordinary fastand stable sodium-ion storage. NanoEnergy 2019, 56, 502-511.
20. Zhu, H.; Gao, G.; Du, M.; Zhou, J.; Wang, K.; Wu, W.; Chen, X.; Li, Y.; Ma, P.; Dong, W.; Duan, F.; Chen, M.; Wu, G.; Wu, J.; Yang, H.; Guo, S., Atomic-Scale Core/ShellStructure Engineering Induces Precise Tensile Strain to Boost HydrogenEvolution Catalysis. Adv Mater 2018, 30 (26).
21. Liang, X.; Gao, G.; Liu, Y.; Ge, Z.; Leng, P.; Wu, G., Carbonnanotubes/vanadium oxide composites as cathode materials for lithium-ionbatteries. J Sol-Gel Sci Techn 2017, 82 (1), 224-232.
22. Bi, W.; Deng, S.; Tang, H.; Liu, Y.; Shen, J.; Gao, G.; Wu, G.; Atif, M.; AlSalhi, M. S.; Gao, G., Coherent V4+-richV2O5/carbon aerogel nanocomposites for high performance supercapacitors. Sci China Mater 2022, 65 (7), 1797-1804.
23. Sun, W.; Du, Y.; Wu, G.; Gao, G.; Zhu, H.; Shen, J.; Zhang, K.; Cao, G., Constructing metallic zinc-cobalt sulfidehierarchical core-shell nanosheet arrays derived from 2Dmetal-organic-frameworks for flexible asymmetric supercapacitors with ultrahighspecific capacitance and performance. JMater Chem A 2019, 7 (12), 7138-7150.
24. Wu, Y.; Gao, G.; Yang, H.; Bi, W.; Liang, X.; Zhang, Y.; Zhang, G.; Wu, G., Controlled synthesis of V2O5/MWCNT core/shell hybridaerogels through a mixed growth and self-assembly methodology forsupercapacitors with high capacitance and ultralong cycle life. J Mater Chem A 2015, 3 (30),15692-15699.
25. Guo, M.; Zhao, W.; Dou, H.; Gao, G.; Zhao, X.; Yang, X.,Decreasing Ion-Diffusion Barrier Enables Superior Na-Ion Storage by SynergizingHierarchical Architecture and Lattice Distortion. Acs Appl Mater Inter 2019,11 (30), 27024-27032.
26. Bi, W.; Jiang, X.; Li, C.; Liu, Y.; Gao, G.; Wu, G.; Atif, M.; AlSalhi, M.; Cao, G.,Effects of Valence States of Working Cations on the Electrochemical Performanceof Sodium Vanadate. Acs Appl Mater Inter 2022, 14 (17), 19714-19724.
27. Liu, Y.; Guan, D.; Gao, G.; Liang, X.; Sun, W.; Zhang, K.; Bi, W.; Wu, G., Enhanced electrochemical performance of electrospun V2O5nanotubes as cathodes for lithium ion batteries. J Alloy Compd 2017, 726, 922-929.
28. Sun, W.; Gao, G.; Du, Y.; Zhang, K.; Wu, G., A facile strategy for fabricating hierarchicalnanocomposites of V2O5 nanowire arrays on a three-dimensional N-doped grapheneaerogel with a synergistic effect for supercapacitors. J Mater Chem A 2018, 6 (21), 9938-9947.
29. Sun, W.; Ji, X.; Gao, G.; Wu, G., A facile strategy for thesynthesis of graphene/V2O5 nanospheres and graphene/VN nanospheres derived froma single graphene oxide-wrapped VOx nanosphere precursor for hybridsupercapacitors. Rsc Adv 2018, 8 (49), 27924-27934.
30. Wang, H.; Gao, G.; Wu, G.; Zhao, H.; Qi, W.; Chen, K.; Zhang, W.; Li, Y., Fast hydrogen diffusion induced by hydrogen pre-splitfor gasochromic based optical hydrogen sensors. Int J Hydrogen Energ 2019,44 (29), 15665-15676.
31. Qi, W.; Gao, G.; Wu, G.; Wang, H., Flexible gasochromic filmswith favorable high temperature resistance and energy efficiency. Sol Energ Mat Sol C 2019, 195, 63-70.
32. Zhang, Z.; Guan, D.; Gao, G.; Wu, G.; Wang, H., Gasochromic properties of novel tungsten oxide thin filmscompounded with methyltrimethoxysilane (MTMS). Rsc Adv 2017, 7 (65), 41289-41296.
33. Bi, W.; Wu, Y.; Liu, C.; Wang, J.; Du, Y.; Gao, G.; Wu, G.; Cao, G., Gradient Oxygen Vacancies in V2O5/PEDOT Nanocables forHigh-Performance Supercapacitors. ACSAppl Energ Mater 2019, 2 (1), 668-677.
34. Gao, G.; Xue, S.; Wang, H.; Zhang, Z.; Wu, G.; Debela, T. T.; Kang, H. S., Highly ThermallyStable and Transparent WO3-SiO2 Gasochromic Films Obtained by an AutomatedPrinting Method. ACS Sustain. Chem. Eng. 2021, 9 (51), 17319-17329.
35. Wang, J.; Ji, Z.; Xu, X.; Chen, T.; Chen, B.; Gao, G.; Ma, J.; Nie, X.; Xu, X., HybridLithographic Arbitrary Patterning of TiO2 Nanorod Arrays. ACS Omega 2022, 7 (25), 22039-22045.
36. Zhang, S.; Gao, G.; Zhu, H.; Cai, L.; Jiang, X.; Lu, S.; Duan, F.; Dong, W.; Chai, Y.; Du, M., In situ interfacialengineering of nickel tungsten carbide Janus structures for highly efficientoverall water splitting. Sci Bull 2020, 65 (8), 640-650.
37. Bi, W.; Wang, J.; Jahrman, E. P.; Seidler, G. T.; Gao, G.; Wu, G.; Cao, G., Interface Engineering V2O5 Nanofibers for High-Energyand Durable Supercapacitors. Small 2019, 15 (31).
38. Zhang, K.; Gao, G.; Sun, W.; Liang, X.; Liu, Y.; Wu, G., Largeinterlayer spacing vanadium oxide nanotubes as cathodes for high performancesodium ion batteries. Rsc Adv 2018, 8 (39), 22053-22061.
39. Zhang, S.; Gao, G.; Hao, J.; Wang, M.; Zhu, H.; Lu, S.; Duan, F.; Dong, W.; Du, M.; Zhao, Y., Low-ElectronegativityVanadium Substitution in Cobalt Carbide Induced Enhanced Electron Transfer forEfficient Overall Water Splitting. AcsAppl Mater Inter 2019, 11 (46), 43261-43269.
40. Gao, G.; Xue, S.; Wang, H.; Zhang, Z.; Shen, J.; Wu, G.,Medium-scale production of gasochromic windows by sol-gel. J Sol-Gel Sci Techn 2022.
41. Liu, Y.; Gao, G.; Liang, X.; Wu, G., Nanofibers ofV2O5/C@MWCNTs as the cathode material for lithium-ion batteries. J Solid State Electr 2018, 22 (8), 2385-2393.
42. Xue, S.; Gao, G.; Zhang, Z.; Jiang, X.; Shen, J.; Wu, G.; Dai, H.; Xu, Y.; Xiao, Y.,Nanoporous WO3 Gasochromic Films for Gas Sensing. Acs Applied Nano Materials 2021,4 (8), 8368-8375.
43. Zeng, Y.; Gao, G.; Wu, G.; Yang, H., Nanosheet-structuredvanadium pentoxide thin film as a carbon- and binder-free cathode forlithium-ion battery applications. J SolidState Electr 2015, 19 (11), 3319-3328.
44. Wang, J.; Cui, C.; Gao, G.; Zhou, X.; Wu, J.; Yang, H.; Li, Q.; Wu, G., A new method to prepare vanadium oxide nano-urchins as acathode for lithium ion batteries. RscAdv 2015, 5 (59), 47522-47528.
45. Bi, W.; Gao, G.; Wu, Y.; Yang, H.; Wang, J.; Zhang, Y.; Liang, X.; Liu, Y.; Wu, G., Novelthree-dimensional island-chain structured V2O5/graphene/MWCNT hybrid aerogelsfor supercapacitors with ultralong cycle life. Rsc Adv 2017, 7 (12), 7179-7187.
46. Liang, X.; Gao, G.; Jiang, X.; Zhang, W.; Bi, W.; Wang, J.; Du, Y.; Wu, G., Preparation of Hydrophobic PPy Coated V2O5 Yolk-ShellNanospheres-Based Cathode Materials with Excellent Cycling Performance. ACS Appl Energ Mater 2020, 3 (3), 2791-2802.
47. Liang, X.; Gao, G., Research Development of NanostructuredVanadium Oxide as Cathodes for Lithium-ion Batteries. Materials Review 2015, 29 (7A), 1-11,33.
48. Liang, X.; Gao, G.; Wu, G.,Research Development of Vanadium Oxide Serving as Cathode Materials for LithiumIon Batteries. Materials Review 2018, 32 (1A), 12-33,40.
49. Gao, G.; Ji, M.; Zhang, K.; Wu, G., rGO/VNTs as Cathodes forHigh Performance Sodium Ion Batteries with Good Cycling Performance. Electronic Materials Letters 2022, 18 (1), 47-56.
50. Sun, W.; Gao, G.; Zhang, K.; Liu, Y.; Wu, G., Self-assembled 3D N-CNFs/V2O5 aerogels with core/shellnanostructures through vacancies control and seeds growth as an outstandingsupercapacitor electrode material. Carbon2018, 132, 667-677.
51. Wu, Y.; Gao, G.; Wu, G.,Self-assembled three-dimensional hierarchical porous V2O5/graphene hybridaerogels for supercapacitors with high energy density and long cycle life. J Mater Chem A 2015, 3 (5), 1828-1832.
52. Bi, W.; Gao, G.; Wu, G.; Atif, M.; AlSalhi, M. S.; Cao,G., Sodium vanadate/PEDOT nanocables rich with oxygen vacancies for high energyconversion efficiency zinc ion batteries. EnergyStorage Mater 2021, 40, 209-218.
53. Yuan, F.; Gao, G.; Jiang, X.; Bi, W.; Su, Y.; Guo, J.; Bao, Z.; Shen, J.; Wu, G.,Suppressing the metal-metal interaction by CoZn0.5V1.5O4 derived fromtwo-dimensional metal-organic frameworks for supercapacitors. Sci China Mater 2021.
54. Yuan, F.; Gao, G.; Jiang, X.; Bi, W.; Su, Y.; Guo, J.; Bao, Z.; Shen, J.; Wu, G.,Suppressing the metal-metal interaction by CoZn0.5V1.5O4 derived fromtwo-dimensional metal-organic frameworks for supercapacitors. Sci China Mater 2022, 65 (1), 105-114.
55. Sun, W.; Gao, G.; Wu, G.; You, Z., Surface-oxidation-mediatedconstruction of Ppy@VNO/NG core-shell host targeting highly capacitive anddurable negative electrode for supercapacitors. Sci China Mater 2021, 64 (9), 2148-2162.
56. Zhang, Z.; Gao, G.; Wang, H.; Wu, G.; Shen, J.; Zhou, B.; Zhang, Z., Synthesis andApplication to Gasochromics of WO3 Nanostructures Based on Sol-Gel Method andHydrothermal Process. Rare Metal Mat Eng 2016, 45, 354-359.
57. Liang, X.; Gao, G.; Feng, S.; Du, Y.; Wu, G., Synthesis and characterization of carbon supported V2O5nanotubes and their electrochemical properties. J Alloy Compd 2019, 772, 429-437.
58. Liang, X.; Gao, G.; Liu, Y.; Zhang, T.; Wu, G., Synthesis and characterization of Fe-doped vanadiumoxide nanorods and their electrochemical performance. J Alloy Compd 2017, 715, 374-383.
59. Liang, X.; Gao, G.; Wu, G.,Synthesis and characterization of hollow and core-shell structured V2O5microspheres and their electrochemical properties. J Alloy Compd 2017, 725, 923-934.
60. Liang, X.; Gao, G.; Wu, G.; Yang, H., Synthesis andcharacterization of novel hierarchical starfish-like vanadium oxide and theirelectrochemical performance. ElectrochimActa 2016, 188, 625-635.
61. Liang, X.; Gao, G.; Du, Y.; Wang, J.; Sun, W.; Liu, Y.; Zhang, K.; Wu, G., Synthesis and characterization of various V2O5microsphere structures and their electrochemical performance. J Alloy Compd 2018, 757, 177-187.
62. Cen, D.; Ding, Y.; Wei, R.; Huang, X.; Gao, G.; Wu, G.; Mei, Y.; Bao, Z., Synthesis of Metal Oxide/Carbon Nanofibers viaBiostructure Confinement as High-Capacity Anode Materials. Acs Appl Mater Inter 2020,12 (26), 29566-29574.
63. Gao, G.; Wu, G., Synthesis, Structure and Electrochemical Propertiesof Vo(x) Nanosheets Prepared from V2O5 and Carbon Aerogels. Rare Metal Mat Eng 2016, 45, 315-319.
64. Bi, W.; Jahrman, E.; Seidler, G.; Wang, J.; Gao, G.; Wu, G.; Atif, M.; AlSalhi, M.; Cao, G.,Tailoring Energy and Power Density through Controlling the Concentration ofOxygen Vacancies in V2O5/PEDOT Nanocable-Based Supercapacitors. Acs Appl Mater Inter 2019, 11 (18), 16647-16655.
65. Dou, Y.; Liang, X.; Gao, G.; Wu, G., Template-free synthesis ofporous V2O5 yolk-shell microspheres as cathode materials for lithium ionbatteries. J Alloy Compd 2018, 735, 109-116.
66. Wang, Q.; Liang, X.; Liu, B.; Song, Y.; Gao, G.; Xu, X.,Thermal conductivity of V2O5 nanowires and their contact thermal conductance. Nanoscale 2020, 12 (2), 1138-1143.
67. Wang, H.; Gao, G.; Wu, G.; Zhang, Z.; Shen, J.; Zhou, B.,TiO2-doped WO3 Gasochromic Thin Films Produced by Sol-Gel Technique with HighHydrogen-sensing Properties. Rare MetalMat Eng 2016, 45, 325-331.
68. Hao, J.; Zhuang, Z.; Cao, K.; Gao, G.; Wang, C.; Lai, F.; Lu, S.; Ma, P.; Dong, W.; Liu, T.; Du, M.; Zhu, H.,Unraveling the electronegativity-dominated intermediate adsorption onhigh-entropy alloy electrocatalysts. NatCommun 2022, 13 (1).
69. Bi, W.; Huang, J.; Wang, M.; Jahrman, E. P.; Seidler, G.T.; Wang, J.; Wu, Y.; Gao, G.; Wu, G.; Cao, G.,V2O5-Conductive polymer nanocables with built-in local electric field derivedfrom interfacial oxygen vacancies for high energy density supercapacitors. J Mater Chem A 2019, 7 (30), 17966-17973.
70. Zhu, H.; Zhang, J.; Yanzhang, R.; Du, M.; Wang, Q.; Gao, G.; Wu, J.; Wu, G.; Zhang, M.; Liu, B.; Yao, J.; Zhang, X., WhenCubic Cobalt Sulfide Meets Layered Molybdenum Disulfide: A Core-Shell SystemToward Synergetic Electrocatalytic Water Splitting. Adv Mater 2015, 27 (32), 4752-4759.
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